Just Accepted
Just Accepted
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ArticleCoordination-covalent assembly of distorted W/Cu/S supramolecular cubes with enhanced third-order nonlinear optical responsesJin Chen, Lao-Bang Wang, Fei-Fan Lang*, Meng-Qi Zhou, Yun-Hu Deng, Jian-Ping Lang*
ABSTRACT
Coordination–covalent assembly of ligand-directed distorted W/Cu/S supramolecular cubes enables enhanced third-order nonlinear optical responses in PMMA composite films. -
ArticleDefect-polaron-electric field synergy in a quinary S-scheme heterojunction for ciprofloxacin degradationTianqi Liu, Zhiyi Zhou, Xinge Hu, Xingda An, Pow-Seng Yap, Konstantinos Papadikis*, Graham Dawson*
Graphitic carbon nitride; Quinary nanocomposite; Visible light photocatalysis; Organic pollutant degradation; Photocatalytic mechanism
ABSTRACT
The nanocomposite was constructed to degrade CIP under visible light via the synergistic effect between S-scheme heterojunction and oxygen vacancy. -
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ArticleRoom-temperature pyroelectric crystal based on a neutral iron(III) spin-crossover compoundZi-Xuan Fan, Wei Lu, Zhao-Ping Ni*, Ming-Liang Tong
Pyroelectric; Spin crossover; Iron; Halogen
ABSTRACT
A neutral iron(III) spin-crossover compound exhibits superior room-temperature pyroelectric performance relative to polyvinylidene fluoride (PVDF) and lead zirconate titanate (PZT). -
ArticleDual-channel optical decoupling of photochromism and room-temperature phosphorescence via ground-state charge transfer for non-destructive anti-counterfeitingYang Hua, Chun-Jie Liu, Yang-Tao Yu, Hang-Hang Guo, Ning-Ning Zhang*, Li Li*
Charge-transfer; Electron-transfer; Non-destructive anti-counterfeiting; Room-temperature-phosphorescence; Photochromism
ABSTRACT
This work presents a decoupling strategy via ground-state charge transfer that separates photochromism and RTP into independent optical channels. This approach solves the non-destructive readout problem in PRTP materials and fulfills a key requirement for advanced anti-counterfeiting systems. -
ArticleCation vacancy-enriched Ce1-xO2/Pd with enhanced H* utilization for efficient electrocatalytic hydrodechlorinationYujia Tang, Xiaokun Fan, Kaixuan Zhang, Yuanyuan Sun, Hao Tan, Yukun Zhu*, Lijie Zhang*
Electrocatalytic hydrodechlorination; Chlorinated organic compounds; Pd catalysts; Cationic vacancy; H* utilization efficiency
ABSTRACT
Cation vacancies on CeO2 effectively modulate H* stabilization and promote its utilization, which endows Pd/Ce1-xO2 with high electrocatalytic hydrodechlorination (EHDC) efficiency.
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ArticleSynergistic coupling of built-in electric field and surface plasmon resonance in Bi/VO-Bi2O2CO3 for boosted photocatalytic CO2-to-CO conversionManning Zha, Yuchun Li, Lili Ai*, Rui Sheng, Dianzeng Jia, Nannan Guo, Luxiang Wang*, Chuan Tan
Bi2O2CO3; Oxygen vacancy; Bi; Photocatalysis; CO2 reduction
ABSTRACT
This study constructs Bi-modified oxygen-deficient Bi2O2CO3 heterojunctions to enhance CO2 photoreduction. The investigation of its structural defects and interfacial features constitutes a core aspect of structural chemistry research. -
ArticleUnlocking atomic-level insights into TM-O-Ce bridges in MOFs: DFT-guided d-p-f hybridization and electronic reconfiguration for boosted and sustained hydrogenationLinmeng Wang‡, Juan Chen‡, Jian Hou, Zhiyuan Liu *, Liang Zhang*, Hao Wu*, Hongyi Gao*
Defective MOFs; TM-O-Ce bridges; Descriptor; Electronic state reconfiguration; DFT-guided synthesis
ABSTRACT
For breaking the stability-activity trade-off in SACs, this study innovatively integrates steric hindrance-coupled d-p-f orbital overlap and electronic effect-incorporated localized d orbital modulation. We propose an intrinsic descriptor φ and unveil the electron push-pull mechanism to identify the optimal TM-O-Ce (i.e., Ni-O-Ce) bridge induced by ligand vacancies in Ce based UiO-66, which assists in the rapid synthesis of promising SACs for boosted and sustained hydrogenation. -
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ArticleInterface-engineered hierarchical MXene-derived In2S3/TiO2/Ti3C2 heterostructure with an S-scheme dual charge-transfer pathway for efficient decontamination of structurally diverse waterborne antibioticsDong-Eun Lee, M.V. Jyothirmai, Satyanarayana Moru, Wan-Kuen Jo*, Surendar Tonda*
In2S3; Ti3C2 MXene; S-scheme mechanism; Antibiotic degradation; Water purification
ABSTRACT
Hierarchical MXene-derived In2S3/TiO2/Ti3C2 heterostructure with an S-scheme charge-transfer pathway enables efficient solar-driven degradation of structurally diverse antibiotics through enhanced charge separation and reactive species generation. -
ArticleS-scheme Al6Si2O13/ZnWO4 nanocomposites for photocatalytic degradation of dichlorvos and triazophos/chlorpyrifos mixturesJinlei Ye, Guoyuan Xiong, Zuhan Wang, Zhen Li*, Jinfeng Zhang*
Organophosphorus pesticides; Solar light; Photocatalysts; S-scheme
ABSTRACT
The S-scheme ASO/ZWO interfacial structure promotes built-in-field-driven charge separation for efficient DDVP and TAP/CPF photodegradation. -
ArticleBaM2Si7As12 (M = Ga, In): Arsenide infrared nonlinear optical crystals via an adding phase strategyShusen Yang, Xuemei Shi, Bingxuan Li, Guang Peng, Ning Ye*, Jindong Chen*
SHG; Adding phase; Nonlinear optical; Arsenides; Tetrahedral ordering
ABSTRACT
Two new arsenide nonlinear optical crystals BaGa2Si7As12 and BaIn2Si7As12 were designed via adding phase strategy. -
ReviewRed and near-infrared emission scintillation crystals: Fundamentals and advancementsChunshen Li, Yuexin Zhu, Peng Zhang*
Light output rate; Red-near infrared; γ-ray spectral; Resolution; Scintillation; Detection limit
ABSTRACT
Two machanisms (band-gap energy level regulation and quantum cutting mechanism) of red/NIR-emitting scintillators to regular the emission region and intensity. -
ReviewRecent advances in efficient photocatalytic H2O2 production from materials design and mechanism understanding to future perspectivesYu Jiang, Enguo Xiang, Ting Zhu*, Long Huang*, Jingwei Li, Kessara Seneesrisakul, Ruchun Li*
Photocatalysis; H2O2 production; Fundamental mechanisms; Structure modulation; Active site engineering; Heterojunction
ABSTRACT
This review comprehensively summarizes recent advances in efficient photocatalytic H2O2 production from material design, mechanism understanding to future perspectives. -
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ReviewSwitchable frameworks: Using MOF structural dynamics to achieve high-selectivity sustainable separations for gases and liquid phasesBrij Mohan, Virender Virender, Harish Kumar Sharma, Sandeep Kumar, Ajeet Singh, Armando J.L. Pombeiro, Rakesh Kumar Gupta*, Gurjaspreet Singh*, Wei Sun*
Metal-organic frameworks; Breathing; Structural flexibility; Surface area; Gas and liquid separation
ABSTRACT
Flexible MOFs harness gate opening, breathing, and swelling to deliver tunable, high-selectivity separations across gas and liquid-phase mixtures sustainably and efficiently. -
ArticleA rapidly self-healing emissive europium cluster-based supramolecular framework via solvent-driven hierarchical co-assemblyJianfeng Peng, Wenkang Guo, Zhida Song, Xuejie Zhang, Shuaijun Yang*, Zi-Yi Chen, Xuchuan Jiang*
Supramolecular assembly framework; Europium clusters; Hierarchical co-assembly; Self-healing; Luminescence
ABSTRACT
Through a solvent-driven, mortise-and-tenon strategy, two chiral europium clusters undergo hierarchical co-assembly to form a supramolecular framework that exhibits rapid self-healing, tunable porosity, and high luminescence efficiency. -
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ArticleStrengthening hydrophilicity in covalent-organic frameworks to boost CO2 photoreductionSi-Zhan Feng†, Chong-Jiu Lu†, Ji-Hua Deng*, Tong-Bu Lu, Di-Chang Zhong*
Covalent organic frameworks (COFs); Hydrophilicity-hydrophobicity; CO2 reduction; HCOOH; Photocatalysis
ABSTRACT
This study reveals at the molecular level that enhanced hydrophilicity accelerates electron and proton transfer and boosts CO2 photoreduction. -
ArticlePoisson-like anisotropic deformation in flexible COFs for highly selective hydrocarbon separationSen Liu, Maohuai Wang, Yang Shao, Shuxian Wei, Baojun Wei*, Xiaoqing Lu*
Flexible covalent organic frameworks; Poisson-like anisotropic deformation; Diffusion selectivity; Machine learning; Hydrocarbon separation
ABSTRACT
This study reveals a Poisson-like anisotropic deformation mechanism in flexible COFs, where guest-induced structural transitions optimize pore environments for selective hydrocarbon separation. -
ArticleAntimony-activated switchable radiation recombination in a single zinc-based hybrid halide crystal for multispectral image fusionPeng Gao, Sheng Gao, Haoyu Zhang, Yifan Li, Yameng Chen*, Youchao Wei*, Yongsheng Liu*, Maochun Hong*
Metal halides; Sb3+ doping; White-light emission; NIR luminescence; X-ray scintillators; Image fusion
ABSTRACT
Sb3+ doping structurally tailors exciton dynamics in a 0D zinc halide to achieve switchable multimodal emission for multispectral image fusion. -
ArticleAccelerated water dissociation kinetics by electron-rich hydrous RuO2 for efficient alkaline hydrogen evolution reactionJingmei Min#, Hao Huang#, Xueyan Wu, Yan Lv, Jiaxin Li, Hongmei Zhang, Fei Song, Jixi Guo*, Dianzeng Jia*
Electron transfer; Electron-rich; Hydrous RuO2; Water dissociation; Alkaline HER
ABSTRACT
The catalytic performance of hydrogen evolution reaction (HER) is closely related to the charge distribution on the surface of catalyst. Developing an electron-enriched catalyst is highly desirable to promote interfacial charge transfer for efficient alkaline HER. Herein, we unveiled that the electron-rich hydrous RuO2 (H-RuO2) supported on MoC@NC plays an essential role in enhancing the HER activity mechanism. -
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![Recent progress on thiacalix[4]arene-stabilized atomically precise metal nanoclusters for photothermal conversion 2026.100978](/Site/default/Uploads/20260512/未标题-3[634].png "Recent progress on thiacalix[4]arene-stabilized atomically precise metal nanoclusters for photothermal conversion 2026.100978")
ReviewRecent progress on thiacalix[4]arene-stabilized atomically precise metal nanoclusters for photothermal conversionDong-Ao Mao, Chong Huang, Wei-Yang Li*, Kun Zhou, Yan-Feng Bi*
Metal nanoclusters; Photothermal conversion; Thiacalix[4]arene; Polyoxometalate
ABSTRACT
Overview of TC4A-supported atomically precise metal nanoclusters for photothermal conversion, with emphasis on design strategies, structure-property relationships, and photothermal conversion mechanisms. -
Bismuth-based S-scheme heterojunctions for efficient photocatalytic energy conversion and applicationWenbo Zheng, Xianfeng Qiao, Shuo Wang, Ying Wang*, Zhengxin Ding*, Jinlin Long*
S-scheme heterojunctions; Bismuth-based catalysts; Photocatalysis; Environmental application
ABSTRACT
This review summarizes recent advances in Bi-based S-scheme heterojunctions, covering charge-transfer mechanisms, construction methods, characterization techniques, modulation strategies, and photocatalytic applications in hydrogen evolution, CO2 reduction, pollutant degradation and H2O2 generation. -
ReviewStructure-function relationships in metal-ligand coordination sensors for metal-ion detectionBrij Mohan*, Ismayil M. Garazade, Khayala Seyidova, Matlab Khamiyev, M.Fátima C. Guedes da Silva, Armando J.L. Pombeiro, Wei Sun*
Preorganized ligands; Supramolecular cages; Coordination polymers; MOFs; Metal ion detection
ABSTRACT
Structure-guided metal–ligand coordination sensors integrate donor selection, coordination geometry, and supramolecular interactions to control selective metal-ion recognition and signal transduction. -
ArticleSynthesis and optical properties of supramolecular uranium(IV) halide complexesXiuru Li†, Yumin Wang†, Junren Wang, Junyi Li, Kai Li,* Zhifang Chai, Shuao Wang, Yaxing Wang*
Supramolecular actinide halides; Uranium(IV) halide complexes; Uranium(IV) photophysics; Decay dynamics
ABSTRACT
First supramolecular actinide halide, (18C6@K)2UCl6, isolates [UCl6]2- octahedra in a 0D lattice, enabling tunable 5f-6d photophysics. -
ArticleUnveiling the Jahn-Teller effect in the excited-state dynamics of Te4+ in 0D Cs2ScCl5·H2O for cryogenic temperature sensingWei Zhang#, Junxiang Liu#, Chenyin Zheng, Zhiqing Shao, Hao Zhang, Dengfeng Yang, Xia Mao, Ping Huang, Xueyuan Chen*, Wei Zheng*
Tellurium; Jahn-Teller effect; Excited-state dynamics; Fluorescent lifetime thermometry; Cryogenic temperature
ABSTRACT
A new fluorescence lifetime thermometric method is developed using Te4+-doped Cs2ScCl5·H2O, enabling cryogenic sensing with a maximum relative sensitivity of 8.5% K–1 at 10 K. -
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ArticleCation-sulfur-driven dimensional reduction engineering for tai-loring sulfonate birefringent crystals with enhanced anisotropyHanjing Huang, Longyun Xu*, Wenli Zhao, Huijian Zhao, Xianghao Kong, Ning Ye, Zhanggui Hu, Conggang Li*
Birefringent crystals; Sulfonate; Dimension engineering
ABSTRACT
Cation-sulfur-driven structural evolution from quasi-2D to quasi-1D triggers a significant birefringence enhancement, exceeding widely used commercial birefringent crystals.
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ArticlePoly (triazine imide) single crystals with chlorine-terminated facets enable chlorine-tolerant photocatalytic seawater splittingWei Xu, Xiaosheng Dang, Qian Wang, Yidong Hou*, Masakazu Anpo, Guigang Zhang*
Photocatalysis; Seawater splitting; Poly (triazine imide); Chlorine tolerance; Ion-framework interaction
ABSTRACT
Poly (triazine imide) crystals with chlorine-terminated facets repel Cl- while attracting Na+, creating an interfacial field that enhances charge separation and prolongs carrier lifetimes for photocatalytic seawater splitting. -
ArticleHigh-crystalline g-C3N4/BiOIO3 S-scheme heterojunction for efficient photocatalytic CO2 reductionZhiyuan Qin#, Haosheng Li#, Song Li, Heng Yang, Juntao Yan, Qiang Ma*, Xiaofang Li*
BiOIO3; High-crystalline g-C3N4; S-scheme heterojunction; Photocatalysis; CO2 reduction
ABSTRACT
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ArticleAnions-mediated interfacial-water regulation boosts C2+ selectivity for CO2 electroreduction over Cu-based catalystsTingting Gong, Zhen Liu, Wen Jin, Jiamei Li, Min Wang*, Luhua Jiang*
CO2 electrochemical reduction; Cu-based catalysts; Interfacial water; Anions; In-situ ATR-SEIRAS
ABSTRACT
Low-concentration anions in 1 M KOH elevate the strong interfacial-water structure proportion following F⁻ > Cl⁻ > Br⁻ > NO3⁻, yielding a volcano relation between C2+ selectivity and strongly hydrogen-bonded water fraction.
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ArticleSulfur-vacancy engineered SmCoO3/MnCdS S-scheme heterojunction for efficient photothermal-photocatalytic H2 evolutionYuanjin He, Hao Yang, Qiwei Guo, Bo Zhou, Xuqiang Hao*, Zhiliang Jin
S-scheme heterojunction; Photocatalytic hydrogen evolution; Vacancy engineering; Photothermal effect; Charge separation
ABSTRACT
A sulfur-vacancy engineered SmCoO3/MnCdS-Vs S-scheme heterojunction with photothermal effect was successfully constructed for boosting photocatalytic hydrogen evolution. -
ArticleModification of structure and electrical properties of antiperovskite Ni3FeN under high pressureTao Han, Yijie Zeng, Pengfei Tan, Meihuan Zhao, Yuxuan Liu, Man-Rong Li*
Antiperovskite nitride; High pressure; Structural phase transition; Electrical transport; Mechanical properties
ABSTRACT
High pressure induces a cubic-to-orthorhombic structural transition in Ni3FeN, accompanied by anomalous resistance rise and mechanical softening, revealing the intrinsic connection between crystal structure evolution and its electrical transport and mechanical behavior. -
ArticleBoosting H2S conversion with S-scheme Cd0.5Zn0.5S/TiO2 nanotube arrays photoanodeWenqi Wang, Xiajie Zhang, Ting Gao, Lin Ju*, Dongqiu Zhao*, Enzhou Liu*
Photoelectrocatalyst; H2S conversion; Cd0.5Zn0.5S; TiO2 nanotube; S-scheme heterojunction
ABSTRACT
S-scheme Cd0.5Zn0.5S/TiO2 nanotube photoanode enables efficient photoelectrocatalytic H2S splitting to H2 and sulfur. -
ReviewAdvances in copper-based catalysts for selective CO₂ electroreduction to C1 and C2 productsShen Wang, Yi Wei, Weijie Li, Chao Han*
CO2 electroreduction; Copper-based catalysts; Selectivity; Stability
ABSTRACT
This work elucidates key descriptors and mechanistic pathways governing Cu-based catalysts for selective CO2 reduction to C1/C2 products, highlighting design strategies and stability challenges. -
ArticleSynergistic modulation of steric hindrance and isomerization space for enhanced photo-regulated performance of metal-organic polyhedraShu Shi†, Mu-Yi Xu†, Yang Liu, Yu-Xia Li, Lin-Bing Sun*
ABSTRACT
Synopsis: Synergistic steric hindrance and isomerization space in (tBu-Azo)(LA)MOP enable efficient solid-state photoisomerization under UV/visible light. -
ArticleDefect-enhanced charge separation in ZnCdS/WS2 S-scheme heterojunctions: Engineering sulfur vacancies to facilitate photocatalytic H2 productionTuo Guo, Guojing Hu, Jiaxin Liu, Li Chen, Guangmin Ren*, Qingjie Guo*
Vs-WS2; ZnCdS; S vacancy; Photocatalytic hydrogen evolution; S-scheme heterojunction
ABSTRACT
Synergistic internal electric field and sulfur vacancies in S-scheme ZnCdS/Vs-WS2 heterojunction enable ultrahigh photocatalytic H2 evolution. -
ArticleAlkoxy chain-length engineering in heterometallic In-Sn-oxo clusters for nanolithographyZhaoke Jin, Weizhou Chen, Yifan Hou, Yuting Ye, Xiuzhen Wang, Xiaofeng Yi*, Jian Zhang*
In-Sn-oxo-clusters; Atomically precise structures; Tunable alkoxy chain-length; Solution processability; Nanolithography
ABSTRACT
This study reveals the critical role of ligands chain length in heterometallic In-Sn-oxo clusters, showing how precise ligand engineering controls solution behavior and patterning mechanism, ultimately unlocking high-resolution lithographic performance. -
ArticleBoosting efficient electrocatalytic CO2 reduction by two-dimensional polyoxometalate@metal-organic framework composites with asymmetric sitesTeng-Fei Yao, Guo-Ping Yang*, Yao-Yu Wang
Polyoxometalates; Metal-organic frameworks; Asymmetric coordination sites; Electrocatalytic CO2 reduction reaction
ABSTRACT
Two Ag-based POM@MOF composites with asymmetric bifunctional sites were synthesized. They synergistically activate CO2 and promote *COOH formation, thereby enhancing electrocatalytic CO2 reduction. -
Hetero-motif POM molecular junctions enable tandem olefin epoxidation and CO2 fixationYingjie Li, Hailong Hu, Aoqi Wang, Jingru Huang, Shiqi Fu, Zongyin Gao, Shuo Tao, Yalin Zhang*, Qingde Zhang*, Haitao Wang, Xianqiang Huang*
Polyoxometalates; Bifunctional catalysis; Olefin epoxidation; CO2 fixation
ABSTRACT
Hetero-motif POM junctions enable synergistic catalysis for olefin epoxidation and CO2 fixation via dual active sites, achieving efficient tandem conversion. -
ArticleMetal-incorporated polymeric resists with tunable lithographic performance via complex-specific designXi Liang, Mei-Hua Xiong, Er-Xia Chen, Lu-Yao Hao, Jin-Xia Yang*, Jian Zhang*, Qipu Lin*
Non-chemically amplified resists; electron-beam lithography; organometal-incorporated polymers; EUV lithography; negative-tone photoresists
ABSTRACT
A new class of sulfonium-centered cationic polymers functionalized with monometallic Sn, Sb, or Bi complexes—denoted BP-Sn, BP-Sb, and BP-Bi—is introduced as non-chemically amplified negative-tone photoresists alongside a metal-free analogue (BP). Maintaining nearly identical backbones and varying only the metal center enables precise control over organometal-specific effects, allowing direct comparative assessment of how Sn, Sb, and Bi govern key lithographic parameters. Systematic investigation reveals distinct performance profiles: BP-Sb achieves the highest sensitivity, BP-Bi delivers superior resolution, and BP-Sn exhibits the sharpest contrast. -
ReviewRecent progress on multi-synergistic charge-transfer strategies for efficient triplet up-conversion in narrowband MR-TADF emittersZeng-Jiang Yue, Zheng-Yin Du*, Xunwen Xiao*, Xu-Feng Luo*
Multiple-resonance; Thermally activated delayed fluorescence; CT modulation; Synergistic channel interactions; OLED
ABSTRACT
This review summarizes multi-synergistic charge-transfer strategies in MR-TADF materials, highlighting how precise structural modulation of excited states enables efficient triplet up-conversion for narrowband OLEDs. -
Spin-state switching driven by divergent structural evolutions in a 3D spin-crossover materialMeng-Ling Wu†, Jun-Hui Liang†, Yan-Ru Chen, Kang Chen, Ze-Yu Ruan, Si-Guo Wu*, Wei-Zhao Cai*, Ming-Liang Tong*
Spin crossover; Pressure; Symmetry breaking; Stimuli-responsive; Spin-state regulation
ABSTRACT
A cyanide-bridged bimetallic coordination polymer featuring one-dimensional zigzag Ag chains with argentophilic interactions was synthesized, and exhibited divergent structural evolutions and spin-state regulation in response to thermal and pressure stimuli. -
ArticleUltramicroporous metal-incorporated HOF with tailored pore confinement for high-efficiency C2H2/CO2 sieving separationYingzhi He, Guangzu Xiong, Wenlei Yang, Yunjia Jiang, Jianbo Hu, Lingyao Wang, Chaoqun Bian*, Yuanbin Zhang*
ABSTRACT
An ultramicroporous metal-incorporated HOF with tailored pore confinement was prepared for high-efficiency C2H2/CO2 sieving separation with benchmark dynamic separation factors. -
Tuning effective conjugation via B←N orientation: High-mobility n-type isoindigo polymers for organic field-effect transistorsJingshu Tian, Haofeng Sun, Jiarui Li, Cheng Wang, Kun Yang, Qinqi Zhou, Kai-kai Liu*, Maning Liu*, Haichang Zhang*
B←N coordination chemistry; n-type conjugated polymers; Organic field-effect transistors (OFETs); Electron mobility; Backbone conformation
ABSTRACT
The vertical configuration of the B←N-coordinated units is conducive to backbone planarity and ordered molecular packing, consequently improving the electron transport mobility in OFETs. -
ArticleMixing enthalpy-induced monodispersed Pb-Zr dual-atomic catalysts for efficient photocatalytic hydrogen peroxide productionWei Zhang#, Dan Liu#, Haishan Zhu#, Longzhou Jin, Shijie Li*, Fang Yang, Yihong Zhang*, Chunqiang Zhuang*
H2O2 production; Dual atom; Mixing enthalpy; Oxygen reduction reaction
ABSTRACT
Mixing enthalpy-driven PbZr dual-atom photocatalyst for efficient photocatalytic oxygen reduction
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